Journal article
Enzymatic carbon dioxide capture using a thermally stable carbonic anhydrase as a promoter in potassium carbonate solvents
G Hu, KH Smith, NJ Nicholas, J Yong, SE Kentish, GW Stevens
Chemical Engineering Journal | ELSEVIER SCIENCE SA | Published : 2017
Abstract
Carbon capture and storage (CCS) is an effective way to reduce CO2 emissions and to mitigate climate change effects. However, the cost of carbon capture has to be reduced to manageable levels before it can be deployed at an industrial scale. Potassium carbonate solutions (K2CO3) are good solvents for CO2 capture because they have low regeneration energy, low degradation rates and low corrosivity. However, one shortcoming of K2CO3 is that it has slow reaction kinetics with CO2. This limitation can be overcome by the addition of promoters to K2CO3 solutions. In this study, the catalysis kinetics of a carbonic anhydrase (NZCA) promoter was tested via the stopped flow technique and a wetted wall..
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Funding Acknowledgements
The authors acknowledge the financial support provided by the Australian Government through its Cooperative Research Center program for this CO2CRC research project. Infrastructure support from the Particulate Fluids Processing Center (PFPC), a Special Research Center of the Australian Research Council is gratefully acknowledged. Peter Cook Centre (PCC) for Carbon Capture and Storage (CCS) Research is also gratefully acknowledged.